Storch starred as Charles Duffy in the TV series The Queen and I in 1969. In 1975 he starred as Eddie Spenser in the series The Ghost Busters. He has voiced roles for The Batman/Superman Hour, Groovie Goolies, The Pink Panther Show, Koko the Clown, Treasure Island, Scooby Doo, and Tennessee Tuxedo. Storch was the first actor to voice The Joker character in Batman. In 1967 he was nominated for a Primetime Emmy Award for F Troop.